Precise control over the generation of intense, ultrafast changes in magnetic fields called “magnetic steps” has been achieved by researchers in Hamburg, Germany. Using ultrashort laser pulses, Andrea Cavalleri and colleagues at the Max Planck Institute for the Structure and Dynamics of Matter disrupted the currents flowing through a superconducting disc. This alters the superconductor’s local magnetic environment on very short timescales – creating a magnetic step.
Magnetic steps rise to their peak intensity in just a few picoseconds, before decaying more slowly in several nanoseconds. They are useful to scientists because they rise and fall on timescales far shorter than the time it takes for materials to respond to external magnetic fields. As a result, magnetic steps could provide fundamental insights into the non-equilibrium properties of magnetic materials, and could also have practical applications in areas such as magnetic memory storage.
So far, however, progress in this field has been held back by technical difficulties in generating and controlling magnetic steps on ultrashort timescales. Previous strategies have employed technologies including microcoils, specialized antennas, and circularly polarized light pulses. However, each of these schemes offer a limited degree of control over the properties of the magnetic steps they generated.
Quenching supercurrents
Now, Cavalleri’s team has developed a new technique that involves the quenching of currents in a superconductor. Normally, these “supercurrents” will flow indefinitely without losing energy, and will act to expel any external magnetic fields from the superconductor’s interior. However, if these currents are temporarily disrupted on ultrashort timescales, a sudden change will be triggered in the magnetic field close to the superconductor – which could be used to create a magnetic step.
To create this process, Cavalleri and colleagues applied ultrashort laser pulses to a thin, superconducting disc of yttrium barium copper oxide (YBCO), while also exposing the disc to an external magnetic field.
To detect whether magnetic steps had been generated, they placed a crystal of the semiconductor gallium phosphide in the superconductor’s vicinity. This material exhibits an extremely rapid Faraday response. This involves the rotation of the polarization of light passing through the semiconductor in response to changes in the local magnetic field. Crucially, this rotation can occur on sub-picosecond timescales.
In their experiments, researchers monitored changes to the polarization of an ultrashort “probe” laser pulse passing through the semiconductor shortly after they quenched supercurrents in their YBCO disc using a separate ultrashort “pump” laser pulse.
“By abruptly disrupting the material’s supercurrents using ultrashort laser pulses, we could generate ultrafast magnetic field steps with rise times of approximately one picosecond – or one trillionth of a second,” explains team member Gregor Jotzu.
Broadband step
This was used to generate an extremely broadband magnetic step, which contains frequencies ranging from sub-gigahertz to terahertz. In principle, this should make the technique suitable for studying magnetization in a diverse variety of materials.
To demonstrate practical applications, the team used these magnetic steps to control the magnetization of a ferrimagnet. Such a magnet has opposing magnetic moments, but has a non-zero spontaneous magnetization in zero magnetic field.
When they placed a ferrimagnet on top of their superconductor and created a magnetic step, the step field caused the ferrimagnet’s magnetization to rotate.
For now, the magnetic steps generated through this approach do not have the speed or amplitude needed to switch materials like a ferrimagnet between stable states. Yet through further tweaks to the geometry of their setup, the researchers are confident that this ability may not be far out of reach.
“Our goal is to create a universal, ultrafast stimulus that can switch any magnetic sample between stable magnetic states,” Cavalleri says. “With suitable improvements, we envision applications ranging from phase transition control to complete switching of magnetic order parameters.”
The research is described in Nature Photonics.
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